Preparation and Research Progress of Polymer-based Flexible Conductive Composites

Xingqiang Chen, Suxing Fang, Zhenpin Hou


The development of flexible wearable electronic devices is one of the future directions of technology development. Flexible conductive materials are important supporting materials for wearable electronic devices. Polymer has excellent flexibility, it is an important way to prepare flexible conductor from polymer-based conductive composites. In this paper, the research progress of polymer-based flexible conductive composites is summarized from the aspects of preparation and characterization methods. The key factors to realize flexible conductor are put forward, namely, the maintenance of excellent polymer elasticity and the realization of stable. The design and preparation of the extensible conductor with high elasticity matrix and nanofiller are introduced in detail, and the problems in the current research are summarized.

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Sekitani T, Yokota T, Zschieschang U, et al. Organic nonvolatile Memory transistors for flexible sensor arrays [J]. Science, 2009, 326: 1516-1519.

Benight S J, Wang C, Tok J B H, et al. Stretchable and selfhealing Polymers and devices for electronic skin [J]. Prog. Polym. Sci. , 2013, 38 (12): 1961-1977.

Rogers J A, Someya T, Huang Y. Materials and mechanics for Stretchable electronics [J]. Science, 2010, 327: 1603-1607.

Sekitani T, Noguchi Y, Hata K, et al. A rubberlike stretchable Active matrix using popularity around [J]. Science, 2008,321:1468-1472.

Li Y, Shimizu H. Toward a stretchable, elastic, and electrically Conductive nanocomposite: morphology and properties of poly [Styrene-b- (ethylene-co-butylene) - B-styrene / multiwalled carbon Nanotube composites fabricated by high-shear processing [J].Macromolecules, 2009, 42: 2587-2593.

Li Y, Zhao L, Shimizu H. Electrically conductive Materials with high stretchability and excellent elasticity by a surface Coating method [J]. Macromol. Rapid Commun , 2011,32:289-294.

Song L, Myers A C, Adams J J, et al. Stretchable and reversibly Deformable radio frequency eth based on silver nanowires[J]. ACS Appl. Mater. Interfaces, 2014, 6: 4248-4253.

Fan J A, Yeo W H, Su Y, et al. Fractal design concepts for Stretchable electronics [J]. Nat. Commun , 2014, 5: 163-180.

Shin M K, Oh J, Lima M, et al. Elastomeric conductive composites Based on carbon nanotube forests [J]. Adv. Mater. , 2010,22: 2663-2667.

Wang X, Hu H, Shen Y, et al. Stretchable Ultrahigh tensile strain and stable metallic conductance enabled by prestrained polyelectrolyte nanoplatforms [J]. Adv. Mater. ,2011,23: 3090-3094.

Xu F, Zhu Y. Highly conductive and stretchable silver nanowire[J]. Adv. Mater. , 2012, 24: 5117-5122.

Zhang Y, Sheehan C J, Zhai J, et al. Polymer-embedded carbon Nanotube ribbons for stretchable donor [J]. Adv. Mater. ,2010, 22: 3027-3031.

Zhu Y, Xu F. Buckling of aligned carbon nanotubes as stretchable A new manufacturing strategy [J]. Adv. Mater. , 2012,24: 1073-1077.

Lin L, Liu S, Fu S, et al. Fabrication of highly stretchable Advertising via morphological control of carbon nanotube network[J]. Small, 2013, 9: 3620-3629.

Kim K H, Vural M, Islam M F. Single-walled carbon nanotube Aerogel-based public around [J]. Adv. Mater. , 2011,23:2865-2869.

Hu H, Zhao Z, Wan W, et al. Ultralight and highly compressible Graphene aerogels [J]. Adv. Mater. , 2013, 25: 2219-2223.

Hu H, Zhao Z, Wan W, et al. Polymer / graphene hybrid aerogel With high compressibility, conductivity, and 'sticky' superhydrophobicity[J]. ACS Appl. Mater. Interfaces, 2014, 6:


Zhao L, Li Y, Qiu J, et al. Reactive bonding mediated high Mass loading of individualized single-walled carbon nanotubes in An elastomeric polymer [J]. Nanoscale, 2012, 4: 6613-6621.

Kim T A, Kim H S, Lee S S, et al. Single-walled carbon Nanotube / silicone rubber composites for compliant electrodes [J]. Carbon, 2012,50: 444-449.

Shang S, Gan L, Yuen M C W, et al. Carbon nanotubes based High temperature vulcanized silicone rubber nanocomposite with Excellent elasticity and electrical properties [J]. Composites Part A, 2014, 66: 135-141.

Shang S, Zeng W, Tao X M. High stretchable MWNTs / Urethane guided nanocomposites [J]. J. Mater. Chem., 2011, 21: 7274-7280.

Liu Z F, Fang S, Moura F A, et al. Hierarchically buckled Sheath-core fibers for superelastic electronics, sensors, and Muscle [J]. Science, 2015, 349: 400-404.

Jiang S, Zhang H, Song S, et al. Highly stretchable Fiber from few-walled carbon nanotubes coated on poly (m-phenylene Isophthalamide) polymer core / shell structures [J]. ACS Nano, 2015, 9: 10252-10257.

Ma R, Kang B, Cho S, et al. Extraordinarily high conductivity Of stretchable fibers of polyurethane and silver nanoflowers [J]. ACS Nano, 2015, 9: 10876-10886.

Persano L, Dagdeviren C, Su Y, et al. High performance Piezoelectric devices based on aligned arrays of nanofibers of poly (Vinylidenefluoride-co-trifluoroethylene) [J]. Nat. Commun , 2013,4: 67-88.

Sun B, Long Y Z, Liu S L, et al. Fabrication of curled conduc-ting polymer microfibrous arrays via a novel electrospinning Method for stretchable strain sensors [J]. Nanoscale, 2013,5:7041-7045.

Boland C S, Khan U, Backes C, et al. Sensitive, high-strain, High-rate bodily motion sensors based on graphene- rubber Composites [J]. ACS Nano, 2014, 8: 8819-8830.

Ding H, Zhong M, Kim Y J, et al. Biologically derived soft Conducting hydrogels using heparin-doped polymer networks[J]. ACS Nano, 2014, 8: 4348-4357.

Kujawski M, Pearse J D, Smela E. Elastomers filled with Exfoliated graphite as compliant electrodes [J]. Carbon, 2010,48: 2409-2417.



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